I15-1 Experimental Timings

I15-1 Experimental Timings

Standard Exposure Times

Perkin Elmer 2 (PE2 - Current Detector In Use)

Minimum exposure time: 3 seconds

Standard exposure time: 10 minutes (+2 minutes for robot change/auto filter etc.)

Considerations and extra functionality:

  • Both can have multiple frames (back-to-back, uninterrupted scans) to allow for quick collections over a physical/chemical process or additional time for weakly scattering samples.

  • Presleep times (times between collections) are recommended between scans to allow for the detector to cool down and clear the image. Otherwise you may experience ‘ghost’ features from previous samples, especially if they were strongly scattering.

ARC Detector

We are currently commissioning this detector and will be able to update expected exposure times once we have determined the best operating procedure.

Set-up Times

All experiments, from simple ex-situ experiments to complicated in-situ setups. Timings to setup these experiments should be included in your experimental plan. Below shows the timings of many things that we have to do on the beamline to make sure the beamline is as optimally setup for your experiment as it can be!

Essentials (60 minutes)

  • Detector calibration: 10 minutes

  • Safety inductions: 30 minutes

  • Induction on how to operate the beamline: 10-60 minutes

  • Loading samples onto the beamline: 15 minutes

All of the above is needed for every experiment, meaning that no experiment will start exactly 9am on the starting day. Even if nothing goes wrong, don’t expect to be running your samples before 10:30am, but realistically expect around lunch time.

  • Temperature device alignment: 15 minutes per device

  • Temperature device calibration: 30-180 minutes (see below)

For temperature device use, expect the essential timings + temperature device timings

  • Optics alignment - 1 day (usually prior to your beamtime)

  • Reference cells on the beamline - 60-120 minutes

  • Getting your real cells onto the beamline - 60 minutes

  • Alignment of cells - 60+ minutes (cell dependent)

  • Alignment and calibration of cell - 60 minutes (additional if using temperature device as well)

  • Setup of gas/flow lines - 60 minutes

  • Setup of gas trolley - 60 minutes

  • References - 10 - 60 minutes

Temperature Device

Characteristics

Device

Max temperature* / K

Min temperature* / K

Max ramp rate / K/min

Min ramp rate / K/min

Device

Max temperature* / K

Min temperature* / K

Max ramp rate / K/min

Min ramp rate / K/min

Blower (hot temperature)

800

350

300

1

Cobra (cold temperature)

450

80

60

0.016

Cryostream (cold temperature)

400

100

60

0.016

* - these are the calibrated sample temperatures we can achieve in optimum conditions, they vary on capillary size, air flow, hutch temperature etc.

Ramp rates are applicable in the temperature 200 - 600K ranges for all devices, expect them to slow as they approach the temperature extremes

  • To do a large temperature range i.e., 100 - 800K we will use both the cold and hot temperature devices to achieve this

Calibrations

All temperature devices require a calibration to ensure your sample is at the temperature that you require. Depending on the range that you require, this can take anywhere from an hour to several hours.

We calibrate by either using lead (low temperature) or a Si/Al2O3 mix (high temperature) and measuring it for 2 minutes at determined temperature points. The temperature device will have an offset between the device temperature and sample temperature (can be up to 200K at the extreme temperatures) and therefore the calibration range will have to be beyond the desired sample temperature. We then run Rietveld refinements to obtain the lattice parameters and determine exact temperatures and apply this on the beamline. From this point forward, temperatures input into the scan will be the temperature your sample will be at.

Hot air blower calibration time (full range): 60 minutes

Cobra/cryostream calibration time (full range): 120 minutes